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problems can be very complicated, as shown in the work of P schl et al. [4]. We only touch on o them here in Section 3.2.9. For a single substance, the chemical potential equilibrium requirement reduces to that the vapour pressure of the substance in the gas be equal to an equilibrium value, pve (T ), which, for a plane surface, depends only on temperature. However, aerosol droplets have spherical curved surfaces, and the Kelvin effect states that the equilibrium vapour pressure over a curved liquid surface, radius R, is increased over that for a plane surface, so that pve (R, T )/ pve (T ) = exp(R /R) 1 + R /R where R is de ned in terms of the liquid surface tension, L, and liquid density, L , by R = 2 v L /( L RG T ) (3.2) where v is the molecular weight. For water droplets, R is 1.071 nm at 20 C decreasing to 0.696 nm at 100 C so that the expanded form is generally adequate in Equation (3.1). Because the vapour pressure varies with R, a cloud of water droplets is never in thermodynamic equilibrium and water will evaporate from smaller size droplets to condense on larger sizes, the Ostwald ripening process discussed in Section 3.3.5. Convenient parameterisations of the equilibrium vapour pressure for water are given in Appendix A, and also a vapour pressure for ice at low temperatures. Because that over water is greater than that over ice, water droplets in a mixed cloud will evaporate and condensation take place on ice particles. Again, no equilibration is possible in a mixed water ice cloud. It should also be noted that there are many different forms of ice particles whose condensation is favoured at different temperatures. (3.1) rdlc pdf 417 PDF417 Barcode Creating Library for RDLC Reports | Generate ...
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